Helical ground state and magnetoelectric properties of two-dimensional Nb3Cl8”

Thomas Olsen (Technical U Denmark, Kongens Lyngby)

Sep 25. 2024, 09:00 — 09:20

Two-dimensional Nb3Cl8 has been proposed as a promising  multiferroic material exhibiting ferrovalley coupling and switchanble ferroelectric ground state. Here we show that such ferrovalley coupling is strongly dependent on the magnetic ground state and is absent in the helimagneti state that is predicted to have the lowest energy in DFT. Moreover, it is shown that switching the polar ground state by an  external electric field is dubious due to a complicated polarization profile along the switching path. On the other hand, the compoiund is shown to exhibit a rich phase diagram and undergoes a first order magnteic phase transition (from commensurate non-collinear to long-range spin spiral) when subjected to strong electric fields.

Further Information
Venue:
ESI Boltzmann Lecture Hall
Recordings:
Recording
Associated Event:
Spin-Orbit Entangled Quantum Magnetism (Workshop)
Organizer(s):
Cesare Franchini (U of Vienna)
Vesna Mitrovic (Brown U, Providence)
Leonid Pourovskii (École Polytechnique, Palaiseau)